Dartington College of Arts was a specialist educational institution at Dartington Hall near Totnes in Devon, southwest England, offering education in music and the arts. Courses prepared students for a career in teaching, in partnership with Rolle College of Education, Exmouth, and came to focus on a performative and multi-disciplinary approach to the arts. Its founder Principal was Peter Cox who had been involved as Warden during its former manifestation before becoming a college. It offered tertiary-level courses in postdramatic theatre, music, choreography, visual performance and performance writing. Its teaching staff were all active arts practitioners.

The college was founded in 1961 as a consequence of the original Dartington Hall experiment in rural regeneration. Academic degrees were validated in partnership with the University of Plymouth in 1975.

Dartington College of Arts became part of University College Falmouth on 6 April 2008 and, in 2010, relocated to Falmouth, Cornwall.

In 2020, The Dartington Arts School was established on the site of the former College of the Arts on the Estate of Dartington Hall Trust.